Surreal illustration of a supercapacitor immersed in a crystalline salt solution, emitting energy waves.

Supercharged Supercapacitors: The Power of a Salty Solution

"Could a novel electrolyte mix unlock cheaper, more powerful, and longer-lasting energy storage?"


Supercapacitors are quickly becoming essential to future energy solutions, bridging the gap between batteries and traditional capacitors. Lithium-ion hybrid electrochemical supercapacitors (L-HECS) combine the best of both worlds: high energy density and rapid charging and discharging. The key to unlocking even greater potential lies in improving the electrolyte, the medium that facilitates ion transport. While organic electrolytes offer a wide voltage window, they often fall short in ionic conductivity, cost, and safety. Aqueous electrolytes are safer and more economical but are limited by water's inherent decomposition voltage.

Recently, scientists have explored “water-in-salt” electrolytes to expand the electrochemical stability window (ESW) of aqueous solutions. These electrolytes use high concentrations of salts to bind water molecules tightly, preventing them from breaking down at lower voltages. However, many of these salts are expensive and impractical for widespread use. Researchers are searching for cost-effective alternatives that can deliver similar performance enhancements.

Now, a team has developed a novel lithium/potassium (Li/K) mixed superconcentrated (SC) aqueous electrolyte that significantly enhances the performance of hybrid supercapacitors. This new electrolyte widens the operating voltage, extends the temperature range, and improves the lifespan of these energy storage devices, offering a compelling path toward more efficient and sustainable energy solutions.

How Does This "Salty" Electrolyte Work?

Surreal illustration of a supercapacitor immersed in a crystalline salt solution, emitting energy waves.

The researchers created a superconcentrated solution of lithium acetate and potassium acetate. Unlike previous approaches, this electrolyte uses a combination of two salts to achieve a unique effect. The high concentration of potassium ions (K+) helps to confine water molecules, while the lithium ions (Li+) contribute to the overall charge capacity. This synergistic combination inhibits hydrogen bonding between water molecules, leading to a wider electrochemical stability window of 2.85V.

The superconcentrated electrolyte offers several key advantages:

  • Wider Voltage Window: The electrolyte prevents water decomposition, allowing the supercapacitor to operate at higher voltages (up to 2.5V), increasing energy storage capacity.
  • Extended Temperature Range: The electrolyte remains stable and functional across a broad temperature range (-30°C to 50°C), making the supercapacitor suitable for various climates and applications.
  • Enhanced Stability: The electrolyte promotes the formation of a stable solid-electrolyte-interphase (SEI) analogue on the anode, protecting it from degradation. It also helps to suppress structural damage to the LiMn2O4 (LMO) cathode.
The resulting hybrid supercapacitor, using LMO as the cathode and activated carbon (AC) as the anode, demonstrates impressive performance. It exhibits high capacity (47.5 mAh g-1 at 60°C), excellent capacity retention (nearly 100% after 20,000 cycles at 2.0V), and ultrahigh energy density (77.9 Wh/kg at 60°C).

The Future of Energy Storage is Salty?

This novel Li/K mixed superconcentrated electrolyte represents a significant step forward in aqueous energy storage. By addressing the limitations of traditional aqueous electrolytes, it paves the way for cheaper, safer, and more powerful supercapacitors.

The improved performance characteristics, particularly the wide operating temperature range and long lifespan, make these supercapacitors attractive for various applications, including electric vehicles, portable electronics, and grid-scale energy storage.

While further research and development are needed to optimize the electrolyte and electrode materials, this innovative approach holds great promise for a sustainable energy future.

About this Article -

This article was crafted using a human-AI hybrid and collaborative approach. AI assisted our team with initial drafting, research insights, identifying key questions, and image generation. Our human editors guided topic selection, defined the angle, structured the content, ensured factual accuracy and relevance, refined the tone, and conducted thorough editing to deliver helpful, high-quality information.See our About page for more information.

This article is based on research published under:

DOI-LINK: 10.1016/j.ensm.2018.10.023, Alternate LINK

Title: Li/K Mixed Superconcentrated Aqueous Electrolyte Enables High-Performance Hybrid Aqueous Supercapacitors

Subject: Energy Engineering and Power Technology

Journal: Energy Storage Materials

Publisher: Elsevier BV

Authors: Wenjun Deng, Xusheng Wang, Chunyi Liu, Chang Li, Jitao Chen, Nan Zhu, Rui Li, Mianqi Xue

Published: 2019-07-01

Everything You Need To Know

1

What is a hybrid supercapacitor, and why is it important?

A hybrid supercapacitor combines the benefits of both supercapacitors and batteries, offering high energy density and rapid charging/discharging capabilities. These devices utilize a lithium-ion hybrid electrochemical supercapacitor (L-HECS) design. The performance of the electrolyte is crucial, as it is the medium that facilitates ion transport within the device. The new electrolyte enhances the overall performance.

2

How does this new 'salty' electrolyte work?

The 'salty' electrolyte is a superconcentrated solution of lithium acetate and potassium acetate. The potassium ions (K+) confine water molecules, while the lithium ions (Li+) contribute to charge capacity. This synergistic effect widens the electrochemical stability window to 2.85V. This is achieved by inhibiting hydrogen bonding between water molecules.

3

What are the key advantages of using this new electrolyte?

The new electrolyte's performance improvements lead to several benefits. A wider voltage window (up to 2.5V) enables higher energy storage. The extended temperature range (-30°C to 50°C) makes the supercapacitor suitable for various climates. Enhanced stability, including a stable solid-electrolyte-interphase (SEI) analogue on the anode and suppressed damage to the LiMn2O4 (LMO) cathode, ensures a longer lifespan and more reliable operation.

4

What were the results of using this new electrolyte in a supercapacitor?

Researchers created a hybrid supercapacitor using the Li/K mixed superconcentrated electrolyte, with LiMn2O4 (LMO) as the cathode and activated carbon (AC) as the anode. This design demonstrated high capacity, excellent capacity retention (nearly 100% after 20,000 cycles at 2.0V), and ultrahigh energy density (77.9 Wh/kg at 60°C). These are key metrics for evaluating the performance of energy storage devices.

5

What is the significance of this new electrolyte for the future of energy storage?

The innovative Li/K mixed superconcentrated electrolyte represents a significant advancement in aqueous energy storage. By resolving the constraints of conventional aqueous electrolytes, it facilitates the development of supercapacitors that are more cost-effective, safer, and more powerful. This could lead to more sustainable energy solutions due to its improved voltage, temperature range, and lifespan.

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